A1 Journal article (refereed)
Observation of Collisional De-Excitation Phenomena in Plutonium (2022)


Raggio, A., Pohjalainen, I., & Moore, I. D. (2022). Observation of Collisional De-Excitation Phenomena in Plutonium. Atoms, 10(2), Article 40. https://doi.org/10.3390/atoms10020040


JYU authors or editors


Publication details

All authors or editorsRaggio, Andrea; Pohjalainen, Ilkka; Moore, Iain D.

Journal or seriesAtoms

eISSN2218-2004

Publication year2022

Publication date20/04/2022

Volume10

Issue number2

Article number40

PublisherMDPI AG

Publication countrySwitzerland

Publication languageEnglish

DOIhttps://doi.org/10.3390/atoms10020040

Publication open accessOpenly available

Publication channel open accessOpen Access channel

Publication is parallel published (JYX)https://jyx.jyu.fi/handle/123456789/80817


Abstract

A program of research towards the high-resolution optical spectroscopy of actinide elements for the study of fundamental nuclear structure is currently ongoing at the IGISOL facility of the University of Jyväskylä. One aspect of this work is the development of a gas-cell-based actinide laser ion source using filament-based dispensers of long-lived actinide isotopes. We have observed prominent phenomena in the resonant laser ionization process specific to the gaseous environment of the gas cell. The development and investigation of a laser ionization scheme for plutonium atoms is reported, focusing on the effects arising from the collision-induced phenomena of plutonium atoms in helium gas. The gas-cell environment was observed to greatly reduce the sensitivity of an efficient plutonium ionization scheme developed in vacuum. This indicates competition between resonant laser excitation and collisional de-excitation by the gas atoms, which is likely being enhanced by the very high atomic level density within actinide elements.


Keywordsnuclear physicsplutoniumresearch equipment

Free keywordscollisional de-excitation; actinide elements; resonance laser ionization; gas cell


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Ministry reportingYes

Reporting Year2022

JUFO rating1


Last updated on 2024-03-04 at 17:27