A2 Katsausartikkeli tieteellisessä aikausilehdessä
Strategies for Exploring Functions from Dynamic Combinatorial Libraries (2020)
Jia, C., Qi, D., Zhang, Y., Rissanen, K., & Li, J. (2020). Strategies for Exploring Functions from Dynamic Combinatorial Libraries. ChemSystemsChem, 2(5), Article e2000019. https://doi.org/10.1002/syst.202000019
JYU-tekijät tai -toimittajat
Julkaisun tiedot
Julkaisun kaikki tekijät tai toimittajat: Jia, Chunman; Qi, Dawei; Zhang, Yucang; Rissanen, Kari; Li, Jianwei
Lehti tai sarja: ChemSystemsChem
eISSN: 2570-4206
Julkaisuvuosi: 2020
Volyymi: 2
Lehden numero: 5
Artikkelinumero: e2000019
Kustantaja: Wiley-VCH Verlag
Julkaisumaa: Saksa
Julkaisun kieli: englanti
DOI: https://doi.org/10.1002/syst.202000019
Julkaisun avoin saatavuus: Avoimesti saatavilla
Julkaisukanavan avoin saatavuus: Osittain avoin julkaisukanava
Julkaisu on rinnakkaistallennettu (JYX): https://jyx.jyu.fi/handle/123456789/68693
Tiivistelmä
Dynamic combinatorial chemistry (DCC) is a powerful approach for creating complex chemical systems, giving access to the studies of complexity and exploration of functionality in synthetic systems. However, compared with more advanced living systems, the man‐made chemical systems are still less functional, due to their limited complexity and insufficient kinetic control. Here we start by introducing strategies to enrich the complexity of dynamic combinatorial libraries (DCLs) for exploiting unexpected functions by increasing the species of building blocks and/or templates used. Then, we discuss how dynamic isomerization of photo‐switchable molecules help DCLs increase and alter the systemic complexity in‐situ. Multi‐phase DCLs will also be reviewed to thrive complexity and functionality across the interfaces. Finally, there will be a summary and outlook about remote kinetic control in DCLs that are realized by applying exogenous physical transduction signals of stress, light, heat and ultrasound.
YSO-asiasanat: supramolekulaarinen kemia; kemiallinen synteesi; kompleksisuus
Vapaat asiasanat: chemical complexity; dynamic combinatorial chemistry; kinetic control; noncovalent interactions; supramolecular chemistry
Liittyvät organisaatiot
OKM-raportointi: Kyllä
Raportointivuosi: 2020
JUFO-taso: 1
